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林产化学与工业 ›› 2016, Vol. 36 ›› Issue (6): 107-118.doi: 10.3969/j.issn.0253-2417.2016.06.017

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生物质基含氧化合物加氢脱氧反应的研究进展

张颖, 韩铮, 徐禄江, 傅尧   

  1. 能源材料化学协同创新中心, 中科院城市污染物转化重点实验室, 安徽省生物质洁净 能源重点实验室, 中国科学技术大学 化学系, 安徽 合肥 230006
  • 收稿日期:2016-06-17 出版日期:2016-12-25 发布日期:2016-12-23
  • 作者简介:张颖(1977-),女,陕西西安人,副教授,博士,主要从事生物质催化转化研究工作;E-mail:zhzhying@ustc.edu.cn
  • 基金资助:
    国家自然科学基金资助项目(21572213);国家973计划资助(2012CB215306)

Recent Progress in Hydrodeoxygenation of Biomass-based Oxygenates

ZHANG Ying, HAN Zheng, XU Lu-jiang, FU Yao   

  1. Collaborative Innovation Center of Chemistry for Energy Material, CAS Key Laboratory of Urban Pollutant Conversion, Anhui Province Key Laboratory of Biomass Clean Energy, Department of Chemistry, University of Science and Technology of China, Hefei 230006, China
  • Received:2016-06-17 Online:2016-12-25 Published:2016-12-23

摘要: 在制备生物燃料过程中,降低原料中氧含量并提高氢碳比非常重要,而加氢脱氧反应则是该过程的关键。从加氢脱氧的基元反应出发,着重依据含氧化合物结构差异和催化体系的不同来综述加氢脱氧的研究进展,以期为寻找一种高效、绿色、经济、可持续地将生物质转化为生物燃料的催化体系提供参考。

关键词: 生物质, 木质素, 加氢脱氧, 含氧化合物, 生物燃料

Abstract: In the preparation of the biofuel or biochemical process, reducing the oxygen content of the feedstock and improving hydrogen carbon ratio are very important. The hydrodeoxygenation is the key to this process. With the expect to provide a reference for finding a highly efficient, green, economic and sustainable catalytic system that can convert biomass into biofuel, this paper focused on the elementary reactions of hydrodeoxygenation and reviewed the development of hydrodeoxygenation reaction according to the differences of oxygen-contained compounds' structure and catalytic systems.

Key words: biomass, lignin, hydrodeoxygenation, oxygenate, biofuels

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