林产化学与工业 ›› 2021, Vol. 41 ›› Issue (1): 107-122.doi: 10.3969/j.issn.0253-2417.2021.01.015
收稿日期:
2020-07-23
出版日期:
2021-02-28
发布日期:
2021-03-03
通讯作者:
刘守新
E-mail:liushouxin@126.com
作者简介:
刘守新, 教授, 博士生导师, 研究领域为功能炭材料以及光催化材料; E-mail: liushouxin@126.com基金资助:
Yuhang ZHANG, Wei LI, Chunhui MA, Sha LUO, Shouxin LIU()
Received:
2020-07-23
Online:
2021-02-28
Published:
2021-03-03
Contact:
Shouxin LIU
E-mail:liushouxin@126.com
摘要:
由CO2等温室气体排放带来的全球变暖问题是目前最严峻的环境问题之一。因此,利用多孔炭材料作为其高效吸附材料的研究得到了广泛的关注。系统综述了近年来用于CO2吸附的5种多孔炭材料,即煤/石油焦基活性炭、生物质多孔炭、炭气凝胶、金属有机骨架衍生物和碳纳米材料,以及多孔炭材料主要的4种制备方法(高温炭化与活化法、水热炭化法、溶胶-凝胶法和模板法),并重点讨论其结构与CO2吸附性能的关系;随后对多孔炭材料的孔结构和表面化学性质吸附CO2的机理进行总结。最后,提出多孔炭材料吸附CO2发展过程中尚待解决的问题,并对其未来的发展方向进行了展望。
中图分类号:
张宇航, 李伟, 马春慧, 罗沙, 刘守新. 多孔炭材料吸附CO2研究进展[J]. 林产化学与工业, 2021, 41(1): 107-122.
Yuhang ZHANG, Wei LI, Chunhui MA, Sha LUO, Shouxin LIU. Progress of Research on CO2 Adsorption by Porous Carbon Materials[J]. Chemistry and Industry of Forest Products, 2021, 41(1): 107-122.
表1
多孔炭材料的孔隙性能和CO2吸附容量汇总"
类型1) type | 前驱体 precursor | 比表面积/ (m2·g-1) SBET | 总孔容/ (cm3·g-1) Vtotal | 微孔孔容/ (cm3·g-1) Vmicro | 孔径/nm pore size | 表面改性 surface modifications | CO2吸附容量CO2 uptake2)/ (mmol·g-1) | 参考文献 ref. | |
25 ℃ | 0 ℃ | ||||||||
Ⅰ | 石油焦petroleum coke | 2363 | 1 | 0.88 | — | 无none | 4.13 | 6.24 | [ |
Ⅱ | 樟脑/山茶花叶 camphor/camellia leaves | 1823 | 1.07 | 0.70 | 2.17 | N(2.15%) | 8.30 | [ | |
柳絮poplar catkins | 1455 | 0.68 | 0.47 | <1.00 | N(2.89%) | 4.05 | 6.22 | [ | |
菱角壳water chestnut shell | 2412 | 1.14 | 0.84 | <1.00 | N(3.14%) | 4.50 | 6.04 | [ | |
枣片date sheet | 2367 | 1.15 | 0.83 | 0.70-0.90 | 无none | 4.36 | 6.40 | [ | |
菱角water chestnut | 3401 | 2.50 | 1.87 | 2.94 | N(4.89%) | 4.70 | 6.00 | [ | |
甘蔗渣sugarcane bagasse | 1113 | 0.57 | 0.51 | 0.55 | N(1.89%) | 4.80 | [ | ||
花生废料peanut waste | 1283 | 0.69 | 0.58 | <0.8 | 无none | 4.24 | 5.33 | [ | |
杉树皮fir bark | 1377 | 0.74 | 0.51 | <0.7 | N(1.00%) | 5.20 | 7.00 | [ | |
桂圆壳longan shells | 3260 | 2.60 | 1.30 | 3.2 | N(2.33%) | 4.30 | 5.60 | [ | |
芦竹Arundo donax | 1863 | 1.00 | — | 2.1 | N(5.40%) | 2.10 | 3.60 | [ | |
葡萄糖D-glucose | 1734 | 0.78 | 0.62 | <1.00 | N(9.24%) | 4.26 | 6.70 | [ | |
烂草莓rotten strawberries | 1117 | 0.52 | 0.39 | <1.00 | N(5.38%) | 4.49 | 6.35 | [ | |
Ⅲ | 间苯二酚/三聚氰胺 resorcinol/melamine | 609 | 0.37 | 0.23 | 2.25 | N(2.50%) | 2.70 | [ | |
间苯二酚/甲醛 resorcinol/formaldehyde | 1871 | 2.03 | 0.77 | 0.8-1.3 | 无none | 3.00 | [ | ||
纤维cellulose | 1364 | 1.42 | 0.37 | — | 无none | 3.42 | [ | ||
纤维cellulose | 615 | 0.64 | 0.21 | — | N(4.62%) | 4.99 | [ | ||
壳多糖chitin | 609 | 521.00 | 0.30 | 0.19 | 无none | 3.44 | 5.02 | [ | |
Ⅳ | bio-MOF-1 | 1129 | 0.55 | 0.40 | — | N(10.16%) | 3.29 | 4.75 | [ |
MIL-100AL | 1097 | 0.82 | 0.49 | — | O(39.50%) | 4.80 | 6.50 | [ | |
Ⅴ | 氧化石墨烯graphene oxide | 13 | 0.03 | 0.01 | — | O(17.20%) | 0.75 | [ | |
氧化石墨烯graphene oxide | 1032 | 0.82 | 0.61 | < 1.00 | N(2.59%) | 2.40 | 3.24 | [ | |
聚多巴胺polydopamine | 561 | — | — | < 0.70 | N(11.60%) | 3.91 | 4.43 | [ |
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