多孔炭材料吸附CO2研究进展

doi:10.3969/j.issn.0253-2417.2021.01.015

Abstract

Abstract:

Global warming caused by greenhouse gas emissions is a pressing environmental problem. Given that CO₂ is the most significant greenhouse gas, research into materials that can efficiently adsorb CO₂ has attracted considerable attention. Compared with other adsorption materials, porous materials offer a large specific surface area with high chemical and thermal stabilities and also feature good adsorption capacity, selectivity, cyclicity, and fast adsorption kinetics; therefore, they are widely used as solid adsorbents for CO₂ capture. This review systematically introduces five types of porous carbon materials coal/petroleum-coke-activated carbons, biomass porous carbons, carbon aerogels, metal-organic-framework-derived carbons, and carbon nanomaterials that have been developed in recent years. Furthermore, the four primary methods used to prepare these materials for CO₂ adsorption (i.e., high temperature carbonization and activation, hydrothermal carbonization, sol-gel processing and the template method) are presented. Emphasis is placed on their structure-performance relationship with CO₂ adsorption. Simultaneously, the mechanism whereby CO₂ is adsorbed by porous carbons with a pore texture is reviewed, in addition to the surface chemistry. Lastly, current challenges pertaining to CO₂ adsorption are summarized, and future development trends are also prospected.

Key words: CO₂ adsorption, porous carbon, solid adsorbent, mechanism

CLC Number:

TQ35
O647.3

Yuhang ZHANG, Wei LI, Chunhui MA, Sha LUO, Shouxin LIU. Progress of Research on CO₂ Adsorption by Porous Carbon Materials[J]. Chemistry and Industry of Forest Products, 2021, 41(1): 107-122.

Figures/Tables 9

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Table 1

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类型¹⁾ type	前驱体 precursor	比表面积/ (m²·g^-1) S_BET	总孔容/ (cm³·g^-1) V_total	微孔孔容/ (cm³·g^-1) V_micro	孔径/nm pore size	表面改性 surface modifications	CO₂吸附容量CO₂ uptake²⁾/ (mmol·g^-1)		参考文献 ref.
类型¹⁾ type	前驱体 precursor	比表面积/ (m²·g^-1) S_BET	总孔容/ (cm³·g^-1) V_total	微孔孔容/ (cm³·g^-1) V_micro	孔径/nm pore size	表面改性 surface modifications	25 ℃	0 ℃	参考文献 ref.
Ⅰ	石油焦petroleum coke	2363	1	0.88	—	无none	4.13	6.24	[11]
Ⅱ	樟脑/山茶花叶 camphor/camellia leaves	1823	1.07	0.70	2.17	N(2.15%)	8.30		[12]
	柳絮poplar catkins	1455	0.68	0.47	<1.00	N(2.89%)	4.05	6.22	[21]
	菱角壳water chestnut shell	2412	1.14	0.84	<1.00	N(3.14%)	4.50	6.04	[13]
	枣片date sheet	2367	1.15	0.83	0.70-0.90	无none	4.36	6.40	[16]
	菱角water chestnut	3401	2.50	1.87	2.94	N(4.89%)	4.70	6.00	[19]
	甘蔗渣sugarcane bagasse	1113	0.57	0.51	0.55	N(1.89%)	4.80		[14]
	花生废料peanut waste	1283	0.69	0.58	<0.8	无none	4.24	5.33	[15]
	杉树皮fir bark	1377	0.74	0.51	<0.7	N(1.00%)	5.20	7.00	[54]
	桂圆壳longan shells	3260	2.60	1.30	3.2	N(2.33%)	4.30	5.60	[55]
	芦竹Arundo donax	1863	1.00	—	2.1	N(5.40%)	2.10	3.60	[56]
	葡萄糖D-glucose	1734	0.78	0.62	<1.00	N(9.24%)	4.26	6.70	[57]
	烂草莓rotten strawberries	1117	0.52	0.39	<1.00	N(5.38%)	4.49	6.35	[58]
Ⅲ	间苯二酚/三聚氰胺 resorcinol/melamine	609	0.37	0.23	2.25	N(2.50%)	2.70		[27]
	间苯二酚/甲醛 resorcinol/formaldehyde	1871	2.03	0.77	0.8-1.3	无none	3.00		[26]
	纤维cellulose	1364	1.42	0.37	—	无none	3.42		[29]
	纤维cellulose	615	0.64	0.21	—	N(4.62%)	4.99		[28]
	壳多糖chitin	609	521.00	0.30	0.19	无none	3.44	5.02	[59]
Ⅳ	bio-MOF-1	1129	0.55	0.40	—	N(10.16%)	3.29	4.75	[33]
Ⅳ	MIL-100AL	1097	0.82	0.49	—	O(39.50%)	4.80	6.50	[34]
Ⅴ	氧化石墨烯graphene oxide	13	0.03	0.01	—	O(17.20%)	0.75		[38]
	氧化石墨烯graphene oxide	1032	0.82	0.61	< 1.00	N(2.59%)	2.40	3.24	[40]
	聚多巴胺polydopamine	561	—	—	< 0.70	N(11.60%)	3.91	4.43	[45]

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Progress of Research on CO₂ Adsorption by Porous Carbon Materials

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Progress of Research on CO₂ Adsorption by Porous Carbon Materials