Chemistry and Industry of Forest Products ›› 2024, Vol. 44 ›› Issue (1): 138-148.doi: 10.3969/j.issn.0253-2417.2024.01.018
Bin LIU1,2(), Songlin ZUO1,*(), Jinlong LIU2
Received:
2022-11-15
Online:
2024-02-28
Published:
2024-02-23
Contact:
Songlin ZUO
E-mail:liubin_nj@126.com;zslnl@njfu.edu.cn
CLC Number:
Bin LIU, Songlin ZUO, Jinlong LIU. Research Progress on the Safety of Activated Carbon in Gas Phase Adsorption Process[J]. Chemistry and Industry of Forest Products, 2024, 44(1): 138-148.
Table 1
Oxidation of various organic compounds on the carbon bed at different temperatures[12-13]"
有机物 organic compound | 125 ℃炭床氧化情况bed oxidation at 125 ℃ | 100 ℃炭床氧化情况bed oxidation at 100 ℃ | |||||||
ΔT/℃ | CO/(mg·g-1) | HST/min | HSP/cm | ΔT/℃ | CO/(mg·g-1) | HST/min | HSP/cm | ||
丙酮acetone | 3 | 0.025 | |||||||
丁酮methyl ethyl ketone | 33 | 1.4 | 7 | 0.2 | |||||
甲基异丁基甲酮 methyl isobutyl ketone | 15 | 0.75 | 4 | 0.06 | |||||
二乙酮diethyl ketone | >200 | >10 | 62 | 86 | 11 | 0.28 | |||
乙基丁酮ethylbutyl ketone | >200 | >10 | 75 | 81 | 6 | 0.275 | |||
二异丁酮diisobutyl ketone | >200 | >10 | 145 | 90 | 4 | 0.08 | |||
环己酮cyclohexanone | >200 | >10 | 5 | 20 | >200 | >10 | 82 | 46 | |
乙酰丙酮diacetone alcohol | >200 | >10 | 3 | 23 | |||||
乙醛acetaldehyde | 6 | 0.03 | |||||||
丙醛propionaldehyde | 30 | 1.7 | 29 | 2.2 | |||||
丁醛butyraldehyde | >200 | >10 | 4 | 70 | >200 | >10 | 60 | 85 | |
醋酸acetic acid | 6 | 0.03 | |||||||
丙酸propanoic acid | >200 | >10 | 17 | 80 | 4 | 0.08 | |||
丁酸butyric acid | >200 | >10 | 21 | 80 | 6 | 0.13 | |||
环己烷cyclohexane | 0 | 0.002 5 | |||||||
丁醇butanol | 0 | 0.005 | |||||||
丁内酯butyrolactone | 0 | 0.015 | |||||||
甲酸甲酯methyl acetate | 0 | 0.005 | |||||||
甲氧基乙醇methyl cellosolve | 0 | 0.021 | |||||||
四氢呋喃tetrahydrofuran | 0 | 0.005 | |||||||
碳carbon | 0 | 0.005 |
Table 2
Comparison of reactivity trends of activated carbon adsorbing organic compound[12-14]"
溶剂 solvent | SRIT/K | RS, 403 K/mW | ΔH/(kJ·mol-1) | 时间/min time | 位置/cm position | 温升/K temp. rise | COmax/(mg·g-1) |
甲苯toluene | 453 | 0 | 167.5 | ||||
乙烷hexane | 451 | 0 | 154.9 | ||||
丙酮acetone | 398 | 0.05 | 104.7 | 3 | 0.025 | ||
丁酮methyl ethyl ketone | 349 | 2.0 | 309.8 | 33 | 2.7 | ||
环己酮cyclohexanone | 338 | 20 | 2 286.0 | 5 | 20 | >200 | >10 |
Table 3
Effect of air flow rate on spontaneous ignition temperature and ignition position[17]"
空气air/(dm3·min-1) | 正常流向normal orientation | 反转方向inverted orientation | |||
SIT/℃ | 着火位置position of ignition | SIT/℃ | 着火位置position of ignition | ||
0.5 | 360 | 底部(空气进入) bottom(air entry) | 465 | ||
1.0 | 325 | 中部middle | 370 | 顶部(空气进入) top(air entry) | |
1.5 | 315 | 中部middle | |||
2.0 | 305 | 顶部(空气出口) top(air exit) | 315 | 底部(空气流出) bottom(air exit) | |
3.0 | 305, 290, 310 (平均mean 303) | 顶部top | |||
3.5 | 310, 300 (平均mean 305) | 顶部top | |||
4.0 | 305, 300 (平均mean 303) | 顶部top | |||
5.0 | 315 | 顶部top | |||
7.0 | 315 | 顶部top | 310 | 底部bottom | |
10.0 | 315 | 顶部top | |||
15.0 | 310, 320, 300 (平均mean 310) | 顶部top | 320 | 底部bottom |
Table 4
Initial oxidation activity of various activated carbons adsorption MEK[14]"
活性炭型号 activated carbon model | 活性炭原料 activated carbon raw material | SRIT/K | RS, 403 K/mW | ΔH/(kJ·mol-1) |
Witco 965 | 沥青petroleum | 383 | 0.6 | 218 |
Witco JXC | 沥青petroleum | 378 | 0.7 | 209 |
Takeda Shirasagi S | 酸洗椰壳coconut-acid washed | 371 | 1.0 | 306 |
Calgon Carbon BPL | 无烟煤smokeless coal | 349 | 2.0 | 310 |
Calgon Carbon CP-IVA | 无烟煤smokeless coal | 343 | 2.3 | 293 |
Norit Sorbonorit B3 | 褐煤peat | 332 | 3.5 | >837 |
Norit Sorbonorit B4 | 褐煤peat | 329 | 3.2 | >837 |
Calgon Carbon PCB | 椰壳coconut shell | 331 | 6.6 | >837 |
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